Search results for "PHOTOINDUCED MAGNETIZATION"

showing 2 items of 2 documents

On/Off Photoswitching in a Cyanide-Bridged {Fe2Co2} Magnetic Molecular Square

2013

International audience; A repeatable bidirectional paramagnetic ↔ diamagnetic photomagnetic effect has been observed in the cyanide-bridged Fe-Co square complex {[Fe{B(pz)(4)}(CN)(3)](2)[Co(bik)(2)](2)}(ClO(4))(2)*3H(2)O [B(pz)(4) = tetrapyrazolylborate, bik = bis(1-methylimidazol-2-yl)ketone]. Magnetic measurements and low-temperature single-crystal X-ray diffraction experiments have shown that a complete electron transfer from the diamagnetic Fe(II)-Co(III) state to the paramagnetic Fe(III)-Co(II) metastable state is induced by 808 nm laser light irradiation, whereas the diamagnetic state is recovered in an almost quantitative yield under irradiation at 532 nm.

CyanideINDUCED ELECTRON-TRANSFERTRANSITIONSRELAXATION010402 general chemistryPhotochemistry01 natural sciencesBiochemistryCOBALT-IRON CYANIDECatalysisPHOTOINDUCED MAGNETIZATIONParamagnetismchemistry.chemical_compoundElectron transferColloid and Surface ChemistryMetastability[SDV.BBM]Life Sciences [q-bio]/Biochemistry Molecular BiologyIrradiationALKALI-METAL-IONPRUSSIAN BLUE ANALOGS010405 organic chemistryChemistryRelaxation (NMR)Photomagnetic effectGeneral Chemistry3. Good health0104 chemical sciencesCOSOLID-STATECrystallographyDiamagnetismJournal of the American Chemical Society
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Prussian Blue Analogues of Reduced Dimensionality

2012

Abstract: Mixed-valence polycyanides (Prussian Blue analogues) possess a rich palette of properties spanning from room-temperature ferromagnetism to zero thermal expansion, which can be tuned by chemical modifications or the application of external stimuli (temperature, pressure, light irradiation). While molecule-based materials can combine physical and chemical properties associated with molecular-scale building blocks, their successful integration into real devices depends primarily on higher-order properties such as crystal size, shape, morphology, and organization. Herein a study of a new reduced-dimensionality system based on Prussian Blue analogues (PBAs) is presented. The system is …

LANGMUIR-BLODGETT-FILMSMaterials scienceSpin glassORDERING TEMPERATUREsingle-chain magnetsNanotechnologyiron(ii) complex02 engineering and technologyCrystal structure010402 general chemistrySINGLE-CHAIN MAGNETSlangmuir-blodgett-films01 natural sciencesThermal expansionBiomaterialsCrystalchemistry.chemical_compoundPHOTOINDUCED MAGNETIZATIONTHIN-FILMSDEGREES-Cphotoinduced magnetizationMoleculeGeneral Materials ScienceCRYSTAL-STRUCTURESThin filmPrussian bluePhysicsGeneral Chemistry021001 nanoscience & nanotechnologyIRON(II) COMPLEX0104 chemical sciencesHYBRID FILMSordering temperaturesquare grid networkChemistrychemistryFerromagnetismSQUARE GRID NETWORKthin-filmshybrid filmsdegrees-c0210 nano-technologyEngineering sciences. Technologycrystal-structuresBiotechnologySmall
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